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The behavior of gain versus peak power deposition and the gain-length product
versus total energ deposited are measured for devices with power deposition levels
from 1 to 13 MW/cm under a variety of gas mixtures. The temporal correlation
between the power deposition and gain shows that both the fluorescence and the gain
occur after the power deposition has concluded for excitation pulses in the range of
10-30 ns. We find that both B-X and C-A fluorescence takes place in the afterglow
and their temporal shapes are similar. This indicates that the C and B states are
tightly coupled. This tight coupling has two detrimental consequences for C-state
lasing. First is that the population of the B and C states are approximately equal
rather than 90 % in the C state believed to exist for short pulse electron beam
excitation. We believe this close coupling is due to the presence of electric fields
in the afterglow which keep the electron temperature relatively hot. The relative
populations of the B and C states are determined by a Boltzman distribution governed
by the electron temperature and their relative energy separation. Second is that
with the C state lifetime approximately the same as the B state lifetime the C-A
saturation intensity is very high and efficient energy extraction is substantially
more difficult.
Robert C. Sze,Marc L. Sentis, andMatteo Vannini
"Time-resolved gain/loss studies under low- and high-power loading for the XeF C-A transition", Proc. SPIE 1278, Excimer Lasers and Applications II, (1 August 1990); https://doi.org/10.1117/12.20613
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Robert C. Sze, Marc L. Sentis, Matteo Vannini, "Time-resolved gain/loss studies under low- and high-power loading for the XeF C-A transition," Proc. SPIE 1278, Excimer Lasers and Applications II, (1 August 1990); https://doi.org/10.1117/12.20613