Population transfer by stimulated Raman scattering with delayed pulses: the concept, some problems, and experimental demonstration

Klaas Bergmann; S. Schiemann; Andreas Kuhn

doi:10.1117/12.58145

1 April 1992 Population transfer by stimulated Raman scattering with delayed pulses: the concept, some problems, and experimental demonstration

Klaas Bergmann, S. Schiemann, Andreas Kuhn

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Proceedings Volume 1638, Optical Methods for Time- and State-Resolved Chemistry; (1992) https://doi.org/10.1117/12.58145
Event: OE/LASE '92, 1992, Los Angeles, CA, United States

Abstract

We discuss recent progress in the attempt to gain complete control over the internal state population of atoms and molecules for collision dynamic studies and spectroscopy. We describe a method which relies on stimulated Raman scattering with pulses delayed in a counter-intuitive way. This method allows highly efficient transfer of population between atomic or molecular levels. It allows, in particular, selective population of highly excited vibrational levels.

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Klaas Bergmann, S. Schiemann, and Andreas Kuhn "Population transfer by stimulated Raman scattering with delayed pulses: the concept, some problems, and experimental demonstration", Proc. SPIE 1638, Optical Methods for Time- and State-Resolved Chemistry, (1 April 1992); https://doi.org/10.1117/12.58145

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