Parametric Raman anti-Stokes laser at 503 nm with phase-matched collinear beam interaction of orthogonally polarized Raman components in calcite under 532 nm 20 ps laser pumping

Sergei Smetanin; Michal Jelínek Jr.; Václav Kubeček

doi:10.1117/12.2268410

16 May 2017 Parametric Raman anti-Stokes laser at 503 nm with phase-matched collinear beam interaction of orthogonally polarized Raman components in calcite under 532 nm 20 ps laser pumping

Sergei Smetanin, Michal Jelínek Jr., Václav Kubeček

Author Affiliations +

Proceedings Volume 10228, Nonlinear Optics and Applications X; 102280U (2017) https://doi.org/10.1117/12.2268410
Event: SPIE Optics + Optoelectronics, 2017, Prague, Czech Republic

Abstract

Lasers based on stimulated-Raman-scattering process can be used for the frequency-conversion to the wavelengths that are not readily available from solid-state lasers. Parametric Raman lasers allow generation of not only Stokes, but also anti-Stokes components. However, practically all the known crystalline parametric Raman anti-Stokes lasers have very low conversion efficiencies of about 1 % at theoretically predicted values of up to 40 % because of relatively narrow angular tolerance of phase matching in comparison with angular divergence of the interacting beams. In our investigation, to widen the angular tolerance of four-wave mixing and to obtain high conversion efficiency into the antiStokes wave we propose and study a new scheme of the parametric Raman anti-Stokes laser at 503 nm with phasematched collinear beam interaction of orthogonally polarized Raman components in calcite under 532 nm 20 ps laser pumping. We use only one 532-nm laser source to pump the Raman-active calcite crystal oriented at the phase matched angle for orthogonally polarized Raman components four-wave mixing. Additionally, we split the 532-nm laser radiation into the orthogonally polarized components entering to the Raman-active calcite crystal at the certain incidence angles to fulfill the tangential phase matching compensating walk-off of extraordinary waves for collinear beam interaction in the crystal with the widest angular tolerance of four-wave mixing. For the first time the highest 503-nm anti-Stokes conversion efficiency of 30 % close to the theoretical limit of about 40 % at overall optical efficiency of the parametric Raman anti-Stokes generation of up to 3.5 % in calcite is obtained due to realization of tangential phase matching insensitive to the angular mismatch.

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Sergei Smetanin, Michal Jelínek Jr., and Václav Kubeček "Parametric Raman anti-Stokes laser at 503 nm with phase-matched collinear beam interaction of orthogonally polarized Raman components in calcite under 532 nm 20 ps laser pumping", Proc. SPIE 10228, Nonlinear Optics and Applications X, 102280U (16 May 2017); https://doi.org/10.1117/12.2268410

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KEYWORDS

Raman spectroscopy

Calcite

Crystals

Laser crystals

Picosecond phenomena

Four wave mixing

Phase matching

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