Presentation
10 March 2020 Ultrafast charge transfer in heterostructures of 2D materials (Conference Presentation)
Stefano Dal Conte, Chiara Trovatello, Zilong Wang, Giulio N. Cerullo
Author Affiliations +
Abstract
We use ultrafast spectroscopy to resolve the interlayer charge scattering processes in heterostructures (HS) of two-dimensional materials. In a WSe2/MoSe2 HS we photogenerate intralayer excitons in MoSe2 and observe hole injection in WSe2 on the sub-picosecond timescale, leading to the formation of interlayer excitons. The temperature dependence of the build-up and decay of interlayer excitons provide insights into the coupling mechanisms. In a graphene/WS2 HS we observe ultrafast charge transfer from graphene to the semiconductor. The data are consistent with hot electron/hole transfer, whereby a tail the hot Fermi-Dirac carrier distribution in graphene tunnels through the Schottky barrier into WS2.
Conference Presentation
© (2020) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
Stefano Dal Conte, Chiara Trovatello, Zilong Wang, and Giulio N. Cerullo "Ultrafast charge transfer in heterostructures of 2D materials (Conference Presentation)", Proc. SPIE 11278, Ultrafast Phenomena and Nanophotonics XXIV, 112781B (10 March 2020); https://doi.org/10.1117/12.2544386
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KEYWORDS
Heterojunctions

Ultrafast phenomena

Excitons

Graphene

Spectroscopy

Absorption

Absorption spectroscopy

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