Microscopic analysis of linear and nonlinear electro-optical properties of tellurium

Jörg Hader; Sven C. Liebscher; Jerome V. Moloney; Stephan W. Koch

doi:10.1117/12.2655725

14 March 2023 Microscopic analysis of linear and nonlinear electro-optical properties of tellurium

Jörg Hader, Sven C. Liebscher, Jerome V. Moloney, Stephan W. Koch

Author Affiliations +

Proceedings Volume 12405, Nonlinear Frequency Generation and Conversion: Materials and Devices XXII; 124050D (2023) https://doi.org/10.1117/12.2655725
Event: SPIE LASE, 2023, San Francisco, California, United States

Abstract

We use first principle DFT-based microscopic many-body models to investigate essential electro-optical properties of bulk tellurium. Absorption/gain and spontaneous emission spectra are calculated using the semiconductor Bloch and luminescence equations. High harmonic generation due to off-resonant excitation and its propagation dependence are studied by coupling the microscopic models to a pulse propagator. Limitations due to intrinsic carrier losses via radiative- and Auger-recombination processes are determined solving quantum-Boltzmann type scattering equations. The strong directional- as well as density- and temperature-dependence of the properties is demonstrated.

Conference Presentation

Citation Download Citation

Jörg Hader, Sven C. Liebscher, Jerome V. Moloney, and Stephan W. Koch "Microscopic analysis of linear and nonlinear electro-optical properties of tellurium", Proc. SPIE 12405, Nonlinear Frequency Generation and Conversion: Materials and Devices XXII, 124050D (14 March 2023); https://doi.org/10.1117/12.2655725

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